[{"awards": "1744961 Olesik, John", "bounds_geometry": "POLYGON((161.711586 -77.75758,161.71322740000002 -77.75758,161.7148688 -77.75758,161.71651020000002 -77.75758,161.7181516 -77.75758,161.719793 -77.75758,161.72143440000002 -77.75758,161.7230758 -77.75758,161.72471720000001 -77.75758,161.7263586 -77.75758,161.728 -77.75758,161.728 -77.75784200000001,161.728 -77.758104,161.728 -77.758366,161.728 -77.758628,161.728 -77.75889000000001,161.728 -77.759152,161.728 -77.75941399999999,161.728 -77.759676,161.728 -77.759938,161.728 -77.7602,161.7263586 -77.7602,161.72471720000001 -77.7602,161.7230758 -77.7602,161.72143440000002 -77.7602,161.719793 -77.7602,161.7181516 -77.7602,161.71651020000002 -77.7602,161.7148688 -77.7602,161.71322740000002 -77.7602,161.711586 -77.7602,161.711586 -77.759938,161.711586 -77.759676,161.711586 -77.75941399999999,161.711586 -77.759152,161.711586 -77.75889000000001,161.711586 -77.758628,161.711586 -77.758366,161.711586 -77.758104,161.711586 -77.75784200000001,161.711586 -77.75758))", "dataset_titles": "Elemental composition of individual nanoparticles and fine particles in 28 Taylor Glacier ice core samples 9000 to 44000 yrs BP; Taylor Glacier Atmospheric Mineral Nanoparticles and Microparticles in Antarctic Ice during the last Climatic Cycle", "datasets": [{"dataset_uid": "200426", "doi": "https://doi.org/10.25921/bd1k-mv46", "keywords": null, "people": null, "repository": "NOAA\u0027s National Centers for Environmental Information World Data Service Paleo archive", "science_program": null, "title": "Taylor Glacier Atmospheric Mineral Nanoparticles and Microparticles in Antarctic Ice during the last Climatic Cycle", "url": "https://www.ncei.noaa.gov/access/paleo-search/study/40380"}, {"dataset_uid": "601879", "doi": "10.15784/601879", "keywords": "Antarctica; Cryosphere; Particle Size; Taylor Glacier", "people": "Kutuzov, Stanislav; Gabrielli, Paolo; Olesik, John; Lowry, Greg; Sullivan, Ryan; Carter, Lucas; Lomax-Vogt, Madeleine", "repository": "USAP-DC", "science_program": null, "title": "Elemental composition of individual nanoparticles and fine particles in 28 Taylor Glacier ice core samples 9000 to 44000 yrs BP", "url": "https://www.usap-dc.org/view/dataset/601879"}], "date_created": "Mon, 06 Jan 2025 00:00:00 GMT", "description": "The main goal of this project is to identify and geochemically characterize atmospheric mineral nanoparticles in pre-industrial Antarctic ice during the last climatic cycle. Recent technological and industrial development is introducing a large number of natural and engineered nanoparticles into Earth\u0027s atmosphere. These constitute a concern for human health, mainly due to their high chemical reactivity. While many atmospheric nanoparticle studies have been performed in modern urban environments, there is essentially no information about their occurrence in a pristine pre-industrial atmosphere. This information is critical, as it constitutes an important benchmark for comparison to the modern atmosphere. Information on nanoparticles from the pre-industrial atmosphere can be obtained from atmospheric mineral nanoparticles that are entrapped in remote pre-industrial Antarctic ice covering the last climatic cycles. Mineral nanoparticles can also affect several climatic processes. First, they directly influence the global energy balance by reflecting solar radiation and indirectly influence through changes in cloud formation (and clouds also reflect solar radiation). Second, atmospheric mineral nanoparticles such as iron oxides could have fertilized the oceans, causing blooms of marine phytoplankton that may have drawn part of the atmospheric carbon dioxide into the oceans during glacial ages (the \"biological pump\"). Third, a significant amount of extraterrestrial material entering the Earth atmosphere is thought to be transported to the poles as nanoparticles called \"meteoric smoke\" that form polar stratospheric clouds implicated in changes of the ozone hole. This project aims to establish the natural background of unknown classes of glacial particles whose size is below the detection limit of the conventional dust analyzers. The team will take advantage of ice samples from the \"horizontal ice core\", already extracted from the remote Taylor Glacier (coastal East Antarctica) covering the last ~44,000 years. These ancient samples are particularly suited to project scope because i) a large ice volume is available ii) the team expects to find a markedly different geochemistry between nanoparticles deposited during the last glacial age and during the current interglacial. A set of advanced techniques including Transmission Electron Microscopy, Single Particle Inductively Coupled Plasma Mass Spectrometry (spICP-MS), spICP-Time of Flight MS, and Field Flow Fractionation will be employed to determine mineral nanoparticle sizes, number/volume, and chemical composition. So far, the elemental composition of dust entrapped in polar ice has been mainly determined by Inductively Coupled Plasma Sector Field Mass Spectrometry and it is generally assumed to be descriptive of the coarse aeolian dust fraction. However, project will test whether or not the determined elemental composition is instead mainly linked to the previously unobserved smaller mineral nanoparticle content. Results on nanoparticles will be compared with a set of new experiments of total dust composition measured by Inductively Coupled Plasma Sector Field Mass Spectrometry, using the same ice samples from Taylor Glacier. This award reflects NSF\u0027s statutory mission and has been deemed worthy of support through evaluation using the Foundation\u0027s intellectual merit and broader impacts review criteria.", "east": 161.728, "geometry": "POINT(161.719793 -77.75889000000001)", "instruments": null, "is_usap_dc": true, "keywords": "MICROPARTICLE CONCENTRATION; Taylor Glacier", "locations": "Taylor Glacier", "north": -77.75758, "nsf_funding_programs": "Antarctic Glaciology", "paleo_time": null, "persons": "Olesik, John", "platforms": null, "repo": "NOAA\u0027s National Centers for Environmental Information World Data Service Paleo archive", "repositories": "NOAA\u0027s National Centers for Environmental Information World Data Service Paleo archive; USAP-DC", "science_programs": null, "south": -77.7602, "title": "Atmospheric Mineral Nanoparticles in Antarctic Ice during the last Climatic Cycle", "uid": "p0010492", "west": 161.711586}, {"awards": "0636740 Kreutz, Karl; 0636767 Dunbar, Nelia", "bounds_geometry": "POINT(112.11666 -79.46666)", "dataset_titles": "Microparticle, Conductivity, and Density Measurements from the WAIS Divide Deep Ice Core, Antarctica; Snowpit Chemistry - Methods Comparison, WAIS Divide, Antarctica; Snowpit evidence of the 2011 Puyehue-Cordon Caulle (Chile) eruption in West Antarctica; WAIS Divide Microparticle Concentration and Size Distribution, 0-2400 ka; WAIS Divide Snowpit Chemical and Isotope Measurements, Antarctica; WAIS Divide WDC06A Discrete ICP-MS Chemistry", "datasets": [{"dataset_uid": "609499", "doi": "10.7265/N5K07264", "keywords": "Antarctica; Density; Electrical Conductivity; Glaciers/ice Sheet; Glaciers/Ice Sheet; Ice Core Records; Microparticle Concentration; Physical Properties; WAIS Divide; WAIS Divide Ice Core", "people": "Koffman, Bess; Breton, Daniel; Hamilton, Gordon S.; Kreutz, Karl", "repository": "USAP-DC", "science_program": "WAIS Divide Ice Core", "title": "Microparticle, Conductivity, and Density Measurements from the WAIS Divide Deep Ice Core, Antarctica", "url": "https://www.usap-dc.org/view/dataset/609499"}, {"dataset_uid": "601036", "doi": "10.15784/601036", "keywords": "Antarctica; Chemistry:ice; Chemistry:Ice; Geochemistry; Geochronology; Glaciers/ice Sheet; Glaciers/Ice Sheet; Ice Core Records; Intracontinental Magmatism; IntraContinental Magmatism; Snow Pit; Tephra; WAIS Divide; WAIS Divide Ice Core", "people": "Koffman, Bess; Kreutz, Karl", "repository": "USAP-DC", "science_program": "WAIS Divide Ice Core", "title": "Snowpit evidence of the 2011 Puyehue-Cordon Caulle (Chile) eruption in West Antarctica", "url": "https://www.usap-dc.org/view/dataset/601036"}, {"dataset_uid": "609506", "doi": "10.7265/N5SJ1HHN", "keywords": "Antarctica; Chemistry:ice; Chemistry:Ice; Geochemistry; Glaciers/ice Sheet; Glaciers/Ice Sheet; Isotope; Microparticle Concentration; Snow/ice; Snow/Ice; WAIS Divide; WAIS Divide Ice Core", "people": "Koffman, Bess; Kreutz, Karl", "repository": "USAP-DC", "science_program": "WAIS Divide Ice Core", "title": "WAIS Divide Snowpit Chemical and Isotope Measurements, Antarctica", "url": "https://www.usap-dc.org/view/dataset/609506"}, {"dataset_uid": "601023", "doi": "10.15784/601023", "keywords": "Antarctica; Chemistry:ice; Chemistry:Ice; Geochemistry; Glaciers/ice Sheet; Glaciers/Ice Sheet; Glaciology; Ice Core Records; ICP-MS; Isotope; WAIS Divide; WAIS Divide Ice Core", "people": "Kreutz, Karl", "repository": "USAP-DC", "science_program": "WAIS Divide Ice Core", "title": "WAIS Divide WDC06A Discrete ICP-MS Chemistry", "url": "https://www.usap-dc.org/view/dataset/601023"}, {"dataset_uid": "609620", "doi": "10.7265/N5Q81B1X", "keywords": "Antarctica; Chemistry:ice; Chemistry:Ice; Geochemistry; Glaciers/ice Sheet; Glaciers/Ice Sheet; Glaciology; Ice Core Records; Trace Elements; WAIS Divide; WAIS Divide Ice Core", "people": "Kreutz, Karl; Koffman, Bess", "repository": "USAP-DC", "science_program": "WAIS Divide Ice Core", "title": "Snowpit Chemistry - Methods Comparison, WAIS Divide, Antarctica", "url": "https://www.usap-dc.org/view/dataset/609620"}, {"dataset_uid": "609616", "doi": "10.7265/N5KK98QZ", "keywords": "Antarctica; Dust; Glaciers/ice Sheet; Glaciers/Ice Sheet; Ice Core Records; Paleoclimate; Particle Size; WAIS Divide; WAIS Divide Ice Core", "people": "Koffman, Bess; Kreutz, Karl", "repository": "USAP-DC", "science_program": "WAIS Divide Ice Core", "title": "WAIS Divide Microparticle Concentration and Size Distribution, 0-2400 ka", "url": "https://www.usap-dc.org/view/dataset/609616"}], "date_created": "Tue, 19 Jun 2012 00:00:00 GMT", "description": "This award supports a project to perform continuous microparticle concentration and size distribution measurements (using coulter counter and state-of-the-art laser detector methods), analysis of biologically relevant trace elements associated with microparticles (Fe, Zn, Co, Cd, Cu), and tephra measurements on the WAIS Divide ice core. This initial three-year project includes analysis of ice core spanning the instrumental (~1850-present) to mid- Holocene (~5000 years BP) period, with sample resolution ranging from subannual to decadal. The intellectual merit of the project is that it will help in establishing the relationships among climate, atmospheric aerosols from terrestrial and volcanic sources, ocean biogeochemistry, and greenhouse gases on several timescales which remain a fundamental problem in paleoclimatology. The atmospheric mineral dust plays an important but uncertain role in direct radiative forcing, and the microparticle datasets produced in this project will allow us to examine changes in South Pacific aerosol loading, atmospheric dynamics, and dust source area climate. The phasing of changes in aerosol properties within Antarctica, throughout the Southern Hemisphere, and globally is unclear, largely due to the limited number of annually dated records extending into the glacial period and the lack of a\u003cbr/\u003etephra framework to correlate records. The broader impacts of the proposed research are an interdisciplinary approach to climate science problems, and will contribute to several WAIS Divide science themes as well as the broader paleoclimate and oceanographic communities. Because the research topics have a large and direct societal relevance, the project will form a centerpiece of various outreach efforts at UMaine and NMT including institution websites, public speaking, local K-12 school interaction, media interviews and news releases, and popular literature. At least one PhD student and one MS student will be directly supported by this project, including fieldwork, core processing, laboratory analysis, and data interpretation/publication. We expect that one graduate student per year will apply for a core handler/assistant driller position through the WAIS Divide Science Coordination Office, and that undergraduate student involvement will result in several Capstone experience projects (a UMaine graduation requirement). Data and ideas generated from the project will be integrated into undergraduate and graduate course curricula at both institutions.", "east": 112.11666, "geometry": "POINT(112.11666 -79.46666)", "instruments": "IN SITU/LABORATORY INSTRUMENTS \u003e CHEMICAL METERS/ANALYZERS \u003e ION CHROMATOGRAPHS; EARTH REMOTE SENSING INSTRUMENTS \u003e PASSIVE REMOTE SENSING \u003e PHOTON/OPTICAL DETECTORS \u003e PARTICLE DETECTORS; IN SITU/LABORATORY INSTRUMENTS \u003e PROBES \u003e ELECTRON MICROPROBES; IN SITU/LABORATORY INSTRUMENTS \u003e PHOTON/OPTICAL DETECTORS \u003e SCANNING ELECTRON MICROSCOPES; IN SITU/LABORATORY INSTRUMENTS \u003e SPECTROMETERS/RADIOMETERS \u003e MASS SPECTROMETERS; IN SITU/LABORATORY INSTRUMENTS \u003e CHEMICAL METERS/ANALYZERS \u003e LOPC-PMS; IN SITU/LABORATORY INSTRUMENTS \u003e SPECTROMETERS/RADIOMETERS \u003e ICP-MS; IN SITU/LABORATORY INSTRUMENTS \u003e ICE CORE MELTER; EARTH REMOTE SENSING INSTRUMENTS \u003e PASSIVE REMOTE SENSING \u003e PHOTON/OPTICAL DETECTORS \u003e PARTICLE DETECTORS", "is_usap_dc": true, "keywords": "Ice Core Dust; Tephra; Radiative Forcing; Greenhouse Gas; West Antarctica; Atmospheric Aerosols; Oxygen Isotope; Not provided; WAIS Divide; Snow Pit; Ice Core Chemistry; Microparticle; Wais Divide-project; Microparticles Size; Paleoclimate; LABORATORY; Ice Core Data; Atmospheric Dynamics; Antarctica; FIELD SURVEYS; Ice Core; Trace Elements; FIELD INVESTIGATION; Holocene; Isotope; Snow Chemistry", "locations": "Antarctica; WAIS Divide; West Antarctica", "north": -79.46666, "nsf_funding_programs": "Antarctic Glaciology; Antarctic Glaciology", "paleo_time": "PHANEROZOIC \u003e CENOZOIC \u003e QUATERNARY \u003e HOLOCENE", "persons": "Koffman, Bess; Kreutz, Karl; Breton, Daniel; Dunbar, Nelia; Hamilton, Gordon S.", "platforms": "LAND-BASED PLATFORMS \u003e FIELD SITES \u003e FIELD INVESTIGATION; LAND-BASED PLATFORMS \u003e FIELD SITES \u003e FIELD SURVEYS; Not provided; OTHER \u003e PHYSICAL MODELS \u003e LABORATORY", "repo": "USAP-DC", "repositories": "USAP-DC", "science_programs": "WAIS Divide Ice Core", "south": -79.46666, "title": "Collaborative Research: Microparticle/tephra analysis of the WAIS Divide ice core", "uid": "p0000040", "west": 112.11666}]

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Atmospheric Mineral Nanoparticles in Antarctic Ice during the last Climatic Cycle

1744961

2025-01-06

Olesik, John

Taylor Glacier Atmospheric Mineral Nanoparticles and Microparticles in Antarctic Ice during the last Climatic Cycle	NOAA's National Centers for Environmental Information World Data Service Paleo archive
Elemental composition of individual nanoparticles and fine particles in 28 Taylor Glacier ice core samples 9000 to 44000 yrs BP	USAP-DC

The main goal of this project is to identify and geochemically characterize atmospheric mineral nanoparticles in pre-industrial Antarctic ice during the last climatic cycle. Recent technological and industrial development is introducing a large number of natural and engineered nanoparticles into Earth's atmosphere. These constitute a concern for human health, mainly due to their high chemical reactivity. While many atmospheric nanoparticle studies have been performed in modern urban environments, there is essentially no information about their occurrence in a pristine pre-industrial atmosphere. This information is critical, as it constitutes an important benchmark for comparison to the modern atmosphere. Information on nanoparticles from the pre-industrial atmosphere can be obtained from atmospheric mineral nanoparticles that are entrapped in remote pre-industrial Antarctic ice covering the last climatic cycles. Mineral nanoparticles can also affect several climatic processes. First, they directly influence the global energy balance by reflecting solar radiation and indirectly influence through changes in cloud formation (and clouds also reflect solar radiation). Second, atmospheric mineral nanoparticles such as iron oxides could have fertilized the oceans, causing blooms of marine phytoplankton that may have drawn part of the atmospheric carbon dioxide into the oceans during glacial ages (the "biological pump"). Third, a significant amount of extraterrestrial material entering the Earth atmosphere is thought to be transported to the poles as nanoparticles called "meteoric smoke" that form polar stratospheric clouds implicated in changes of the ozone hole. This project aims to establish the natural background of unknown classes of glacial particles whose size is below the detection limit of the conventional dust analyzers. The team will take advantage of ice samples from the "horizontal ice core", already extracted from the remote Taylor Glacier (coastal East Antarctica) covering the last ~44,000 years. These ancient samples are particularly suited to project scope because i) a large ice volume is available ii) the team expects to find a markedly different geochemistry between nanoparticles deposited during the last glacial age and during the current interglacial. A set of advanced techniques including Transmission Electron Microscopy, Single Particle Inductively Coupled Plasma Mass Spectrometry (spICP-MS), spICP-Time of Flight MS, and Field Flow Fractionation will be employed to determine mineral nanoparticle sizes, number/volume, and chemical composition. So far, the elemental composition of dust entrapped in polar ice has been mainly determined by Inductively Coupled Plasma Sector Field Mass Spectrometry and it is generally assumed to be descriptive of the coarse aeolian dust fraction. However, project will test whether or not the determined elemental composition is instead mainly linked to the previously unobserved smaller mineral nanoparticle content. Results on nanoparticles will be compared with a set of new experiments of total dust composition measured by Inductively Coupled Plasma Sector Field Mass Spectrometry, using the same ice samples from Taylor Glacier. This award reflects NSF's statutory mission and has been deemed worthy of support through evaluation using the Foundation's intellectual merit and broader impacts review criteria.

Collaborative Research: Microparticle/tephra analysis of the WAIS Divide ice core

0636740
0636767

2012-06-19

Koffman, Bess; Kreutz, Karl; Breton, Daniel; Dunbar, Nelia; Hamilton, Gordon S.

Microparticle, Conductivity, and Density Measurements from the WAIS Divide Deep Ice Core, Antarctica	USAP-DC
Snowpit evidence of the 2011 Puyehue-Cordon Caulle (Chile) eruption in West Antarctica	USAP-DC
WAIS Divide Snowpit Chemical and Isotope Measurements, Antarctica	USAP-DC
WAIS Divide WDC06A Discrete ICP-MS Chemistry	USAP-DC
Snowpit Chemistry - Methods Comparison, WAIS Divide, Antarctica	USAP-DC
WAIS Divide Microparticle Concentration and Size Distribution, 0-2400 ka	USAP-DC

This award supports a project to perform continuous microparticle concentration and size distribution measurements (using coulter counter and state-of-the-art laser detector methods), analysis of biologically relevant trace elements associated with microparticles (Fe, Zn, Co, Cd, Cu), and tephra measurements on the WAIS Divide ice core. This initial three-year project includes analysis of ice core spanning the instrumental (~1850-present) to mid- Holocene (~5000 years BP) period, with sample resolution ranging from subannual to decadal. The intellectual merit of the project is that it will help in establishing the relationships among climate, atmospheric aerosols from terrestrial and volcanic sources, ocean biogeochemistry, and greenhouse gases on several timescales which remain a fundamental problem in paleoclimatology. The atmospheric mineral dust plays an important but uncertain role in direct radiative forcing, and the microparticle datasets produced in this project will allow us to examine changes in South Pacific aerosol loading, atmospheric dynamics, and dust source area climate. The phasing of changes in aerosol properties within Antarctica, throughout the Southern Hemisphere, and globally is unclear, largely due to the limited number of annually dated records extending into the glacial period and the lack of a<br/>tephra framework to correlate records. The broader impacts of the proposed research are an interdisciplinary approach to climate science problems, and will contribute to several WAIS Divide science themes as well as the broader paleoclimate and oceanographic communities. Because the research topics have a large and direct societal relevance, the project will form a centerpiece of various outreach efforts at UMaine and NMT including institution websites, public speaking, local K-12 school interaction, media interviews and news releases, and popular literature. At least one PhD student and one MS student will be directly supported by this project, including fieldwork, core processing, laboratory analysis, and data interpretation/publication. We expect that one graduate student per year will apply for a core handler/assistant driller position through the WAIS Divide Science Coordination Office, and that undergraduate student involvement will result in several Capstone experience projects (a UMaine graduation requirement). Data and ideas generated from the project will be integrated into undergraduate and graduate course curricula at both institutions.

USAP-DC